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In some embodiments, the non-naturally occurring microbial organism additional features a 1,three-butanediol pathway comprising no less than one exogenous nucleic acid encoding an enzyme chosen from: 1) Hydrogenase, 2) Carbon monoxide dehydrogenase, 3) Succinyl-CoA transferase, or Succinyl-CoA synthetase (or succinyl-CoA ligase), 4) Succinyl-CoA reductase (aldehyde forming), 5) 4-Hydroxybutyrate dehydrogenase, 6) 4-Hydroxybutyrate kinase, 7) Phosphotrans-4-hydroxybutyrylase, eight) four-Hydroxybutyryl-CoA dehydratase, 9) Crotonase, 10) 3-Hydroxybutyryl-CoA reductase (aldehyde forming), 11) 3-Hydroxybutyraldehyde reductase, 12) Succinate reductase, thirteen) Succinyl-CoA reductase (alcohol forming), 14) 4-Hydroxybutyryl-CoA transferase, or four-Hydroxybutyryl-CoA synthetase, 15) three-Hydroxybutyryl-CoA reductase (alcohol forming), 16) three-Hydroxybutyryl-CoA hydrolase, or 3-Hydroxybutyryl-CoA synthetase, or 3-Hydroxybutyryl-CoA transferase, 17) three-Hydroxybutyrate reductase In some embodiments, the non-naturally occurring microbial organism features a butanol pathway that includes a minimum of one exogenous nucleic acid encoding an enzyme chosen from 1) Hydrogenase, 2) Carbon monoxide dehydrogenase, three) Succinyl-CoA transferase, or Succinyl-CoA synthetase (or succinyl-CoA ligase), four) Succinyl-CoA reductase (aldehyde forming), 5) 4-Hydroxybutyrate dehydrogenase, 6) 4-Hydroxybutyrate kinase, 7) Phosphotrans-four-hydroxybutyrylase, eight) four-Hydroxybutyryl-CoA dehydratase, 9) butyryl-CoA dehydrogenase, 10) Butyryl-CoA reductase (aldehyde forming), eleven) Butyraldehyde reductase, 12) Succinate reductase, 13) Succinyl-CoA reductase (alcohol forming), 14) four-Hydroxybutyryl-CoA transferase, or 4-Hydroxybutyryl-CoA synthetase, 15) Butyryl-CoA reductase (alcohol forming), 16) Butyryl-CoA hydrolase, or Butyryl-CoA synthetase, or Butyryl-CoA transferase, 17) Butyrate reductase. 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